大气腐蚀中液滴覆盖下腐蚀现象的研究方法进展
Research Method Development of Corrosion under Droplets during Atmospheric Corrosion
摘 要
综述了近几十年来国内外对大气腐蚀过程中液滴覆盖下腐蚀现象的研究,尤其是近十年来随着研究手段的发展,对液滴覆盖下的腐蚀有了深入的研究.主要的研究手段有体视显微镜,环境扫描显微镜,Kelvin电极,原子力显微镜以及电化学阻抗谱等方法.这些现代研究方法的采用,使大气腐蚀的研究向原位观测和原子尺度方向发展,同时促进了对液滴覆盖下腐蚀机理的深入研究.
原位观测
液滴
atmospheric corrosion
in-situ monitoring technology
droplet
Abstract
The development of research methods for corrosion under droplets during atmospheric corrosion is reviewed.With the revolution of experimental technology,the corrosion under droplet has been investigated deeply.Main measuring techniques include microscopy,environmental scanning electron microscopy (ESEM),Kelvin probe,atom force microscopy (AFM),electrochemical impedance spectroscopy (EIS) and so on.Using these modern measurements,the mechanism research of corrosion under droplets has been promoted.The development trend of droplet corrosion research will be in-situ monitoring technology and atomic scale observation.
中图分类号 TG172.3 TG174.3
所属栏目 专论
基金项目 国家科技基础条件平台建设项目(2005DKA10400);国家自然科学基金项目(50499331-8)
收稿日期 2009/4/17
修改稿日期 2009/12/25
网络出版日期
作者单位点击查看
备注李磊,博士研究生.
引用该论文: LI Lei,LI Xiao-gang,DONG Chao-fang,XIAO Kui. Research Method Development of Corrosion under Droplets during Atmospheric Corrosion[J]. Corrosion & Protection, 2010, 31(4): 260～264
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参考文献
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【25】Wang Rongguang,Kido Mitsuo.Condensation and evaporation behaviors of micro-water droplets on SUS304 steel observed using the ac noncontact mode of AFM[J].Materials Letters,2003,57(16/17):2360-2365.
【26】Wang Rongguang,Kido Mitsuo.Corrosion behavior of pure iron beneath a micro-droplet of sulfuric acid solution investigated by atomic force microscopy[J].Scripta Materialia,2006,55(7):633-636.
【27】Wang Rongguang,Kido Mitsuo.Corrosion behavior of pure iron by different droplet volume of sulfuric acid solution[J].Materials Transactions,2007,48(6):1451-1457.
【28】Wang Rongguang,Kido Mitsuo.Influence of attractive force on imaging micro-droplets of water by atomic force microscope[J].Surface and Interface Analysis,2005,37(12):1105-1110.
【29】Wang Rongguang,Kido Mitsuo,Suzumura Fumihiro.XPS analysis and atomic force microscopy observation of micro-liquids adsorbed on pure iron and copper surfaces[J].Materials Science Forum,2004,449-452(II):1025-1028.
【30】Wang Rongguang,Kido Mitsuo,Morihiro Naoki.An XPS and atomic force microscopy study of the micro-wetting behavior of water on pure chromium[J].Materials Transactions,2003,44(3):389-395.
【31】Wang Rongguang.An AFM and XPS study of corrosion caused by micro-liquid of dilute sulfuric acid on stainless steel[J].Applied Surface Science,2004,227(3):399-409.
【32】严川伟,何毓番,林海潮,等.铜在含SO2大气中的腐蚀初期规律和机理[J].中国有色金属学报,2000,10(5):645-648.
【33】Kleber Ch,Schreiner M.In situ TM-AFM investigations of the influence of zinc and tin as alloy constituents of copper to the early stages of corrosion[J].Applied Surface Science,2003,217(7):294-301.
【34】Zhang Da-quan,An Zhong-xun,Pan Qing-yi,et al.Volatile corrosion inhibitor film formation on carbon steel surface and its inhibition effect on the atmospheric corrosion of carbon steel[J].Applied Surface Science,2006,253(3):1343-1348.
【35】Kleber Ch,Hilfrich U Schreiner.In situ QCM and TM-AFM investigations of the early stages of degradation of silver and copper surfaces[J].Applied Surface Science,2007,253(7):3712-3721.
【36】Kleber Ch,Hilfrich U,Schreiner M.In situ investigations of the interaction of small inorganic acidifying molecules in humidified air with polycrystalline metal surfaces by means of TM-AFM,IRRAS,and QCM[J].Surface and Interface Analysis,2007,39(8):702-710.
【37】Hu J,Xiao XD,Ogletree D F,et al.Structure of molecularly thin films of water on mica in humid environments[J].Surface Science,1995,344(3):221-236.
【38】Hu J,Xiao XD,Ogletree D F,et al.Atomic scale friction and wear of mica[J].Surface Science,1995,327(3):358-370.
【39】Hu J,Xiao XD,Ogletree D F,et al.Imaging the condensation and evaporation of molecularly thin films of water with nanometer resolution[J].Surface Science,1995,268(4):267-269.
【40】Dubuisson Emilie,Lavie Philippe,Dalard Francis,et al.Study of the atmospheric corrosion of galvanised steel in a micrometric electrolytic droplet[J].Electrochemistry Communications,2006,8(6):911-915.
【41】Chatillon C,Coudurier L,Eustathopoulos N.Corrosion mechanism at the gas-solid-liquid triple line for aluminium droplets on alumina substrates under vacuum[J].Materials Science Forum,2001,369-372(I):263-268.
【2】Barton K.Protection against atmospheric corrosion-theories and methods[C]//London: A Wiley-Interscience Publication,1976.
【3】Evans U R,Taylor C A J.Mechanism of Atmospheric Rusting[J].Corrosion Science,1972,12(3):227-246.
【4】Graedel T E.Gildes model studies of aqueous chemistry.I.Formulation and potential applications of the multi-regime model[J].Corrosion Science,1996,38(12):2153-2180.
【5】肖纪美.腐蚀总论——材料的腐蚀及其控制方法[M].北京:化学工业出版社,1994.
【6】Li Bian,Weng Yongji,Li Xiangyi.Observation of micro-droplets on metal surface in early atmospheric corrosion[J].Electrochemistry Communications,2005,7(10):1033-1038.
【7】Chen Jian,Wang Jianqiu,Ke Wei.In situ observation of formation and spreading of micro-droplets on magnesium and its alloy under cyclic wet-dry condition[J].Corrosion Science,2007,49(3):1625-1634.
【8】林翠.金属材料在典型污染大气环境中初期腐蚀行为和机理研究[D].北京:北京科技大学,博士学位论文,2004.
【9】Stratmann M,Streckel H.On the atmospheric corrosion of metals which are covered with thin electrolyte layers-I.Verification of the experimental technique[J].Corrosion Science,1990,30(6/7):684-696.
【10】Stratmann M,Streckel H.On the atmospheric corrosion of metals which are covered with thin electrolyte layers.II.Experimental results[J].Corrosion Science,1990,30(6/7):697-671.
【11】Stratmann M,Streckel H,Kim K T,et al.On the atmospheric corrosion of metals which are covered with thin electrolyte layers-iii.the measurement of polarisation curves on metal surfaces which are covered by thin electrolyte layers[J].Corrosion Science,1990,30(6/7):715-734.
【12】Frankel G S,Stratmann M,Rohwerder M,et al.Potential control under thin aqueous layers using a Kelvin probe[J].Corrosion Science,2007,49(4):2021-2036.
【13】Neufeld A K,Cole I S,Bond A M,et al.The initiation mechanism of corrosion of zinc by sodium chloride particle deposition[J].Corrosion Science,2002,44(3):555-572.
【14】Tsutsumi Yusuke,Nishikata Atsushi,Tsuru Tooru.Pitting corrosion mechanism of Type 304 stainless steel under a droplet of chloride solutions[J].Corrosion Science,2007,49(3):1394-1407.
【15】Tsuru Tooru,Tamiya Ken-Ichiro,Nishikata Atsushi.Formation and growth of micro-droplets during the initial stage of atmospheric corrosion[J].Electrochimica Acta,2004,49(7):2709-2715.
【16】Zhang J B,Wang J,Wang Y.Micro-droplets formation during the deliquescence of salt particles in atmosphere[J].Corrosion,2005,61(12):1167-1172.
【17】Zhang Jibiao,Wang Jia,Wang Yanhua.Electrochemical investigations of micro-droplets formed on metals during the deliquescence of salt particles in atmosphere[J].Electrochemistry Communications,2005,7(4):443-448.
【18】张际标,王燕华,姜应律,等.微液滴现象与大气腐蚀.I.微液滴的形成与扩展[J].中国腐蚀与防护学报,2006,26(4):207-210.
【19】张际标,王燕华,姜应律,等.微液滴现象与大气腐蚀.II.微液滴现象的电化学表征[J].中国腐蚀与防护学报,2006,26(5):282-285.
【20】王佳.气相环境中无机盐微粒沉积金属表面的电位分布[J].中国腐蚀与防护学报,2004,24(1):1-5.
【21】王佳.无机盐微粒沉积和大气腐蚀的发生与发展[J].中国腐蚀与防护学报,2004,24(3):155-158.
【22】张际标.大气腐蚀起始过程中的微液滴现象研究[D].中国科学院海洋研究所,博士学位论文,2005.
【23】肖葵.典型金属材料大气腐蚀初期行为和机理研究[D].北京:北京科技大学,博士学位论文,2006.
【24】梁丽花.大气腐蚀起始阶段微液滴现象研究[D].青岛:中国海洋大学,硕士学位论文,2006.
【25】Wang Rongguang,Kido Mitsuo.Condensation and evaporation behaviors of micro-water droplets on SUS304 steel observed using the ac noncontact mode of AFM[J].Materials Letters,2003,57(16/17):2360-2365.
【26】Wang Rongguang,Kido Mitsuo.Corrosion behavior of pure iron beneath a micro-droplet of sulfuric acid solution investigated by atomic force microscopy[J].Scripta Materialia,2006,55(7):633-636.
【27】Wang Rongguang,Kido Mitsuo.Corrosion behavior of pure iron by different droplet volume of sulfuric acid solution[J].Materials Transactions,2007,48(6):1451-1457.
【28】Wang Rongguang,Kido Mitsuo.Influence of attractive force on imaging micro-droplets of water by atomic force microscope[J].Surface and Interface Analysis,2005,37(12):1105-1110.
【29】Wang Rongguang,Kido Mitsuo,Suzumura Fumihiro.XPS analysis and atomic force microscopy observation of micro-liquids adsorbed on pure iron and copper surfaces[J].Materials Science Forum,2004,449-452(II):1025-1028.
【30】Wang Rongguang,Kido Mitsuo,Morihiro Naoki.An XPS and atomic force microscopy study of the micro-wetting behavior of water on pure chromium[J].Materials Transactions,2003,44(3):389-395.
【31】Wang Rongguang.An AFM and XPS study of corrosion caused by micro-liquid of dilute sulfuric acid on stainless steel[J].Applied Surface Science,2004,227(3):399-409.
【32】严川伟,何毓番,林海潮,等.铜在含SO2大气中的腐蚀初期规律和机理[J].中国有色金属学报,2000,10(5):645-648.
【33】Kleber Ch,Schreiner M.In situ TM-AFM investigations of the influence of zinc and tin as alloy constituents of copper to the early stages of corrosion[J].Applied Surface Science,2003,217(7):294-301.
【34】Zhang Da-quan,An Zhong-xun,Pan Qing-yi,et al.Volatile corrosion inhibitor film formation on carbon steel surface and its inhibition effect on the atmospheric corrosion of carbon steel[J].Applied Surface Science,2006,253(3):1343-1348.
【35】Kleber Ch,Hilfrich U Schreiner.In situ QCM and TM-AFM investigations of the early stages of degradation of silver and copper surfaces[J].Applied Surface Science,2007,253(7):3712-3721.
【36】Kleber Ch,Hilfrich U,Schreiner M.In situ investigations of the interaction of small inorganic acidifying molecules in humidified air with polycrystalline metal surfaces by means of TM-AFM,IRRAS,and QCM[J].Surface and Interface Analysis,2007,39(8):702-710.
【37】Hu J,Xiao XD,Ogletree D F,et al.Structure of molecularly thin films of water on mica in humid environments[J].Surface Science,1995,344(3):221-236.
【38】Hu J,Xiao XD,Ogletree D F,et al.Atomic scale friction and wear of mica[J].Surface Science,1995,327(3):358-370.
【39】Hu J,Xiao XD,Ogletree D F,et al.Imaging the condensation and evaporation of molecularly thin films of water with nanometer resolution[J].Surface Science,1995,268(4):267-269.
【40】Dubuisson Emilie,Lavie Philippe,Dalard Francis,et al.Study of the atmospheric corrosion of galvanised steel in a micrometric electrolytic droplet[J].Electrochemistry Communications,2006,8(6):911-915.
【41】Chatillon C,Coudurier L,Eustathopoulos N.Corrosion mechanism at the gas-solid-liquid triple line for aluminium droplets on alumina substrates under vacuum[J].Materials Science Forum,2001,369-372(I):263-268.
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