碳点在食品安全检测中的应用
Application of Carbon Dots in Food Safety Detection
摘 要
综述了碳点（CDs）的荧光性质（包括荧光产生机理、激发光/酸度依赖性、化学稳定性、抗光漂白性和上转换荧光）、合成方法（水热合成法、溶剂热法、超声波振荡法和微波消解法），重点讨论了其在食品安全检测中的应用，包括对重金属离子、合法和违禁食品添加剂、农药和兽药残留、食品中营养成分和病原体的检测，并对CDs发展趋势进行了展望（引用文献86篇）。
荧光性质
合成方法
食品安全检测
综述
carbon dot
fluorescence property
synthetic method
food safety testing
review
Abstract
Fluorescence properties of CDs (including fluorescence mechanism, excitation light/acidity dependence, chemical stability, resistance to photobleaching and upconversion fluorescence) and synthetic methods (including hydrothermal synthesis, solvent hot method, ultrasonic oscillation and microwave digestion) were reviewed. The focus was placed on the discussion of its application in the food safety testing, including heavy metal ions, legal and illegal food additives, pesticides and veterinary drug residues, food nutrition and pathogen detection, and the development trend was prospected for CDs (86 ref. cited).
中图分类号 O65 DOI 10.11973/lhjy-hx202105009
所属栏目 综述
基金项目
收稿日期 2020/7/17
修改稿日期
网络出版日期
作者单位点击查看
备注邓晨,硕士,主要从事在食品安全检测方面的应用研究工作
引用该论文: DENG Chen,ZHOU Hualan,LIANG Yingfang,WANG Feng,ZHANG Jianguo. Application of Carbon Dots in Food Safety Detection[J]. Physical Testing and Chemical Analysis part B:Chemical Analysis, 2021, 57(5): 427～435
邓晨,周化岚,梁营芳,王锋,张建国. 碳点在食品安全检测中的应用[J]. 理化检验－化学分册, 2021, 57(5): 427～435
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参考文献
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【5】QU J H, WEI Q, SUN D W. Carbon dots:Principles and their applications in food quality and safety detection[J]. Critical Reviews in Food Science and Nutrition, 2018,58(14):2466-2475.
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【7】DE B, KARAK N. A green and facile approach for the synthesis of water soluble fluorescent carbon dots from banana juice[J]. RSC Advances, 2013,3(22):8286-8290.
【8】GHOSH S, CHIZHIK A M, KAREDLA N, et al. Photoluminescence of carbon nanodots:Dipole emission centers and electron-phonon coupling[J]. Nano Letters, 2014,14(10):5656-5661.
【9】WU M B, WANG Y, WU W T, et al. Preparation of functionalized water-soluble photoluminescent carbon quantum dots from petroleum coke[J]. Carbon, 2014,78:480-489.
【10】GUDE V, DAS A, CHATTERJEE T, et al. Molecular origin of photoluminescence of carbon dots:Aggregation-induced orange-red emission[J]. Physical Chemistry Chemical Physics:PCCP, 2016,18(40):28274-28280.
【11】SONG Y B, ZHU S J, ZHANG S T, et al. Investigation from chemical structure to photoluminescent mechanism:A type of carbon dots from the pyrolysis of citric acid and an amine[J]. Journal of Materials Chemistry C, 2015,3(23):5976-5984.
【12】SCHNEIDER J, RECKMEIER C J, XIONG Y, et al. Molecular fluorescence in citric acid-based carbon dots[J]. The Journal of Physical Chemistry C, 2017,121(3):2014-2022.
【13】DING H, YU S B, WEI J S, et al. Full-color light-emitting carbon dots with a surface-state-controlled luminescence mechanism[J]. ACS Nano, 2016,10(1):484-491.
【14】BAO L, LIU C, ZHANG Z L, et al. Photoluminescence-tunable carbon nanodots:Surface-state energy-gap tuning[J]. Advanced Materials, 2015,27(10):1663-1667.
【15】WANG Y Y, LI Y, YAN Y, et al. Luminescent carbon dots in a new magnesium aluminophosphate zeolite[J]. Chemical Communications, 2013,49(79):9006-9008.
【16】ZHENG B Z, LIU T, PAAU M C, et al. One pot selective synthesis of water and organic soluble carbon dots with green fluorescence emission[J]. RSC Advances, 2015,5(15):11667-11675.
【17】LI Z, YU H J, BIAN T, et al. Highly luminescent nitrogen-doped carbon quantum dots as effective fluorescent probes for mercuric and iodide ions[J]. Journal of Materials Chemistry C, 2015,3(9):1922-1928.
【18】CAI L, FU Z, CUI F. Synthesis of carbon dots and their application as turn off-on fluorescent sensor for mercury(Ⅱ) and glutathione[J]. Journal of Fluorescence, 2020,30(1):11-20.
【19】TONG L L, WANG X X, CHEN Z Z, et al. One-step fabrication of functional carbon dots with 90% fluorescence quantum yield for long-term lysosome imaging[J]. Analytical Chemistry, 2020,92(9):6430-6436.
【20】ZUO P L, LU X H, SUN Z G, et al. A review on syntheses, properties, characterization and bioanaly-tical applications of fluorescent carbon dots[J]. Microchimica Acta, 2016,183(2):519-542.
【21】QIAN Z S, MA J J, SHAN X Y, et al. Highly luminescent N-doped carbon quantum dots as an effective multifunctional fluorescence sensing platform[J]. Chemistry-A European Journal, 2014,20(8):2254-2263.
【22】SHI L H, LI Y Y, LI X F, et al. Controllable synthesis of green and blue fluorescent carbon nanodots for pH and Cu2+ sensing in living cells[J]. Biosensors and Bioelectronics, 2016,77:598-602.
【23】DUTTA C S, CHETHODIL J M, GHARAT P M, et al. pH-elicited luminescence functionalities of carbon dots:Mechanistic insights[J]. The Journal of Physical Chemistry Letters, 2017,8(7):1389-1395.
【24】JIN X Z, SUN X B, CHEN G, et al. pH-sensitive carbon dots for the visualization of regulation of intracellular pH inside living pathogenic fungal cells[J]. Carbon, 2015,81:388-395.
【25】WANG C X, XU Z Z, CHENG H, et al. A hydrothermal route to water-stable luminescent carbon dots as nanosensors for pH and temperature[J]. Carbon, 2015,82:87-95.
【26】JIA X F, LI J, WANG E K. One-pot green synthesis of optically pH-sensitive carbon dots with upconversion luminescence[J]. Nanoscale, 2012,4(18):5572-5575.
【27】MA Z, MING H, HUANG H, et al. One-step ultrasonic synthesis of fluorescent N-doped carbon dots from glucose and their visible-light sensitive photocatalytic ability[J]. New Journal of Chemistry, 2012,36(4):861-864.
【28】PEI S P, ZHANG J, GAO M P, et al. A facile hydrothermal approach towards photoluminescent carbon dots from amino acids[J]. Journal of Colloid and Interface Science, 2015,439:129-133.
【29】LIU M L, CHEN B B, LIU Z X, et al. Highly selective and sensitive detection of 2,4,6-trinitrophenol by using newly developed blue-green photoluminescent carbon nanodots[J]. Talanta, 2016,161:875-880.
【30】WEN X P, SHI L H, WEN G M, et al. Green and facile synthesis of nitrogen-doped carbon nanodots for multicolor cellular imaging and Co2+ sensing in living cells[J]. Sensors and Actuators B:Chemical, 2016,235:179-187.
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