分子印迹荧光探针在农药检测中的应用进展
Application Progress of Molecularly Imprinted Fluorescent Probe in Pesticide Detection
摘 要
分子印迹聚合物由于可特异性地从样品溶液中富集目标物,已被广泛应用于粮食、果蔬等食品以及水、土壤等环境中农药的提取和检测。将分子印迹技术和量子点修饰技术相结合形成的分子印迹荧光探针,可以实现对目标物的高灵敏快速检测。据此,对分子印迹技术的原理、制备方法及应用进行了概述,并进一步阐述了量子点修饰的分子印迹荧光探针在农药检测中的应用和展望。
制备方法
量子点
农药检测
molecularly imprinted polymer
preparation method
quantum dot
pesticide detection
Abstract
The molecularly imprinted polymer could specifically enrich the target compounds from the sample solution, which had been widely used in the extraction and detection of pesticides in food including cereals, fruits and vegetables, and in the environment including water and soil. The molecularly imprinted fluorescent probe formed by combining molecular imprinting technology and quantum dot modification technology could achieve high-sensitivity and rapid detection of the target compounds. Therefore, the principle, preparation method and application of molecular imprinting technology were summarized, and the application and prospect of quantum dot-modified molecularly imprinted fluorescent probe in pesticide detection were further elaborated.
中图分类号 O65 DOI 10.11973/lhjy-hx202206021
所属栏目 综述
基金项目 上海市科委创新行动计划农业领域项目(19391902200)
收稿日期 2021/7/5
修改稿日期
网络出版日期
作者单位点击查看
联系人作者曹慧(caohuian@126.com)
备注王胜洁,硕士研究生,主要从事分子印迹荧光探针在新烟碱类农药快速检测方面的应用研究工作
引用该论文: WANG Shengjie,WEI Ziqi,CAO Hui,XU Fei,YE Tai,YUAN Min,WU Xiuxiu,YIN Fengqin,YU Jinsong,HAO Liling. Application Progress of Molecularly Imprinted Fluorescent Probe in Pesticide Detection[J]. Physical Testing and Chemical Analysis part B:Chemical Analysis, 2022, 58(6): 735～744
王胜洁,魏子奇,曹慧,徐斐,叶泰,袁敏,吴秀秀,阴凤琴,于劲松,郝丽玲. 分子印迹荧光探针在农药检测中的应用进展[J]. 理化检验－化学分册, 2022, 58(6): 735～744
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【7】AHMADPOUR H, HOSSEINI S M M. A solid-phase luminescence sensor based on molecularly imprinted polymer-CdSeS/ZnS quantum dots for selective extraction and detection of sulfasalazine in biological samples[J]. Talanta, 2018,194:534-541.
【8】刘欣,孙秀兰,曹进.分子印迹技术在食品样品安全分析中的应用[J].食品安全质量检测学报, 2020,11(1):106-113.
【9】ASHLEY J, SHAHBAZI M A, KANT K, et al. Molecularly imprinted polymers for sample preparation and biosensing in food analysis:Progress and perspectives[J]. Biosensors and Bioelectronics, 2017,91:606-615.
【10】SONG X Q, ZHOU T, LIU Q Y, et al. Molecularly imprinted solid-phase extraction for the determination of ten macrolide drugs residues in animal muscles by liquid chromatography-tandem mass spectrometry[J]. Food Chemistry, 2016,208:169-176.
【11】MAR AC'G M, KUPKA T, WIECZOREK P P, et al. Computational modeling of molecularly imprinted polymers as a green approach to the development of novel analytical sorbents[J]. Trends in Analytical Chemistry, 2018,98:64-78.
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【14】FARRINGTON K, MAGNER E, REGAN F. Predicting the performance of molecularly imprinted polymers:Selective extraction of caffeine by molecularly imprinted solid phase extraction[J]. Analytica Chimica Acta, 2006,566(1):60-68.
【15】LIU W, GUO Y M, LUO J, et al. A molecularly imprinted polymer based a lab-on-paper chemiluminescence device for the detection of dichlorvos[J]. Spectrochimica Acta, Part A:Molecular and Biomolecular Spectroscopy, 2015,141:51-57.
【16】LUO X P, LI C Z, DUAN Y Q, et al. Molecularly imprinted polymer prepared by Pickering emulsion polymerization for removal of acephate residues from contaminated waters[J]. Journal of Applied Polymer Science, 2016,133(15):43126.
【17】HASHEMI-MOGHADDAM H, JEDI D J. Solid-phase microextraction of chlorpyrifos in fruit samples by synthesised monolithic molecularly imprinted polymer fibres[J]. International Journal of Environmental Analytical Chemistry, 2015,95(1):33-44.
【18】MOTAHARIAN A, MOTAHARIAN F, ABNOUS K, et al. Molecularly imprinted polymer nanoparticles-based electrochemical sensor for determination of diazinon pesticide in well water and apple fruit samples[J]. Analytical and Bioanalytical Chemistry, 2016,408(24):6769-6779.
【19】MARTINS N, CARREIRO E P, SIMOES M, et al. An emerging approach for the targeting analysis of dimethoate in olive oil:The role of molecularly imprinted polymers based on photoiniferter induced "living" radical polymerization[J]. Reactive&Functional Polymers, 2015,86:37-46.
【20】YE T, YIN W X, ZHU N X, et al. Colorimetric detection of pyrethroid metabolite by using surface molecularly imprinted polymer[J]. Sensors&Actuators, B:Chemical, 2018,254:417-423.
【21】LI Y G, ZHANG L, DANG Y Y, et al. A robust electrochemical sensing of molecularly imprinted polymer prepared by using bifunctional monomer and its application in detection of cypermethrin[J]. Biosensors and Bioelectronics, 2018,127:207-214.
【22】QIU H M, LUO C N, SUN M, et al. A novel chemiluminescence sensor for determination of quercetin based on molecularly imprinted polymeric microspheres[J]. Food Chemistry, 2012,134(1):469-473.
【23】CHEN L G, LI B. Determination of imidacloprid in rice by molecularly imprinted-matrix solid-phase dispersion with liquid chromatography tandem mass spectrometry[J]. Journal of Chromatography B:Analytical Technologies in the Biomedical and Life Sciences, 2012,897:32-36.
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