基于声发射技术的锆合金微弧氧化涂层拉伸失效监测
Tensile Failure Monitoring of Zirconium Alloy Micro-arc Oxidation CoatingBased on Acoustic Emission Technology
摘 要
通过恒压微弧氧化设备在锆合金基体表面制备了微弧氧化涂层,运用声发射技术对涂层试样的拉伸过程进行实时监测,通过声发射特征参数的分析与拉伸断口形貌的观察,研究了涂层试样的拉伸失效过程,并运用快速傅里叶变换识别了涂层拉伸失效的频率特征。结果表明:微弧氧化涂层对锆合金拉伸性能的影响主要表现在拉伸过程中的塑性阶段;在拉伸过程中,涂层中的微裂纹随机向各个方向扩展,导致涂层在塑性阶段(132~222 s)发生集中性剥离脱落现象,且试样断裂前涂层已基本从基体上脱落,仅在断口的局部区域零星分布一些不规则形状的涂层;涂层拉伸失效的频率特征是在0.023,0.039,0.055 MHz处出现了3个强烈的信号,并在大于0.8 MHz的频段中出现微弱的稳定信号。
微弧氧化
拉伸失效
声发射技术
涂层
zirconium alloy
micro-arc oxidation
tensile failure
acoustic emission technology
coating
Abstract
The micro-arc oxidation coating was prepared on the surface of zirconium alloy substrate by the constant pressure micro-arc oxidation equipment. The tensile process of the coating sample was monitored in real time by acoustic emission technology. The tensile failure process of the coating sample was studied by analysis of acoustic emission characteristic parameters and observation of tensile fracture morphology, and the frequency characteristics of the coating tensile failure were identified by fast Fourier transform. The results show that micro-arc oxidation coating mainly affected the tensile properties of zirconium alloy at the plastic stage. During the tensile process, the microcracks in the coating randomly extended in all directions, leading to the phenomenon of concentrated peeling of the coating at the plastic stage (132-222 s); the coating was basically detached from the substrate before fracture, and only some irregular coating was scattered in the local area of the fracture. The frequency characteristics of coating tensile failure were three strong signal at 0.023, 0.039, 0.055 MHz, and weak stable signal in the frequency band greater than 0.8 MHz.
中图分类号 TG410.20 DOI 10.11973/jxgccl202206012
所属栏目 专题报道（金属材料表面处理）
基金项目 国家自然科学基金资助项目(U2067221);四川省科技计划项目(2022JDJQ0019)
收稿日期 2021/4/20
修改稿日期 2022/4/27
网络出版日期
作者单位点击查看
备注周腾(1988-),男,浙江诸暨人,博士研究生导师:蔡振兵研究员
引用该论文: ZHOU Teng,CHEN Huan,LI Zhengyang,YUE Yanan,ZHANG Ruiqian,CAI Zhenbing. Tensile Failure Monitoring of Zirconium Alloy Micro-arc Oxidation CoatingBased on Acoustic Emission Technology[J]. Materials for mechancial engineering, 2022, 46(6): 71～77
周腾,陈寰,李正阳,岳雅楠,张瑞谦,蔡振兵. 基于声发射技术的锆合金微弧氧化涂层拉伸失效监测[J]. 机械工程材料, 2022, 46(6): 71～77
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参考文献
【1】SHANKAR A R,RAJU V R,RAO M N,et al.Corrosion of zircaloy-4 and its welds in nitric acid medium[J].Corrosion Science,2007,49(9):3527-3538.
【2】张强,齐世锋,陈鸿飞,等.在高温硝酸与丙烷蒸气环境中R60702工业纯锆的腐蚀行为[J].机械工程材料,2020,44(7):33-37. ZHANG Q,QI S F,CHEN H F,et al.Corrosion behavior of R60702 industrial pure zirconium in high temperature nitric acid and propane vapor[J].Materials for Mechanical Engineering,2020,44(7):33-37.
【3】MOTTA A T, YILMAZBAYHAN A, SILVA M J G D, et al. Zirconium alloys for supercritical water reactor applications:Challenges and possibilities[J]. Journal of Nuclear Materials, 2007, 371(1/2/3):61-75.
【4】GHOSAL S K, PALIT G C, DE P K. Corrosion of zirconium alloys in nuclear applications-A review[J]. Mineral Processing&Extractive Metallurgy Review, 2002, 22(4/5/6):519-546.
【5】NOUDURU S K, MANDAPAKA K K, ROYCHOWDHURY S, et al. Nodular corrosion of zirconium alloys in gaseous environment containing different contaminants[J]. Journal of Nuclear Materials, 2020, 545:152640.
【6】LI Z Y, CAI Z B, CUI X J, et al. Influence of nanoparticle additions on structure and fretting corrosion behavior of micro-arc oxidation coatings on zirconium alloy[J]. Surface and Coatings Technology, 2021, 410:126949.
【7】BRACHET J C, SAUX M L, BISCHOFF J, et al. Evaluation of equivalent cladding reacted parameters of Cr-coated claddings oxidized in steam at 1200℃ in relation with oxygen diffusion/partitioning and post-quench ductility[J]. Journal of Nuclear Materials, 2020,533:152106.
【8】BRAGG-SITTON S. Development of advanced accident tolerant fuels for commercial light water reactors[J]. Nuclear News, 2014, 57(3):83-91.
【9】CHEN H, WANG X, ZHANG R. Application and development progress of Cr-based surface coating in nuclear fuel elements:II. Current status and shortcomings of performance studies[J]. Coatings, 2020, 10(9):835-835.
【10】TANG C, STUEBER M, SEIFERT H J, et al. Protective coatings on zirconium-based alloys as accident-tolerant fuel (ATF) claddings[J]. Corrosion Reviews, 2017, 35(3):141-165.
【11】王晓云,马一林,田林海,等.Al2O3掺杂与超声辅助对纯铝表面微弧氧化层结构与性能的影响[J].机械工程材料,2018,42(11):52-57. WANG X Y,MA Y L,TIAN L H,et al.Effect of Al2O3 doping and ultrasonic assisting on structure and properties of micro-arc oxidation coating on surface of pure aluminum[J].Materials for Mechanical Engineering,2018,42(11):52-57.
【12】LIU F,SHAN D Y,SONG Y W,et al.Corrosion behavior of the composite ceramic coating containing zirconium oxides on AM30 magnesium alloy by plasma electrolytic oxidation[J].Corrosion Science,2011,53(11):3845-3852.
【13】XUE W,WANG C,TIALN H,et al.Corrosion behaviors and galvanic studies of microarc oxidation films on Al-Zn-Mg-Cu alloy[J].Surface&Coatings Technology,2007,201(21):8695-8701.
【14】WANG Y M,JIANG B L,GUO L X,et al.Tribological behavior of microarc oxidation coatings formed on titanium alloys against steel in dry and solid lubrication sliding[J].Applied Surface Science,2006,252(8):2989-2998.
【15】CHENG Y L,CAO J H,PENG Z M,et al.Wear-resistant coatings formed on zircaloy-2 by plasma electrolytic oxidation in sodium aluminate electrolytes[J].Electrochimica Acta,2014,116:453-466.
【16】YANG J, WANG X, WEN Q, et al. The effect of microarc oxidation and excimer laser processing on the microstructure and corrosion resistance of Zr-1Nb alloy[J]. Journal of Nuclear Materials, 2015, 467:186-193.
【17】MATYKINA E, ARRABAL R, SKELDON P, et al. Investigation of the growth processes of coatings formed by AC plasma electrolytic oxidation of aluminium[J]. Electrochimica Acta, 2009, 54(27):6767-6778.
【18】XUE W B,ZHU Q Z,JIN Q,et al.Characterization of ceramic coatings fabricated on zirconium alloy by plasma electrolytic oxidation in silicate electrolyte[J].Materials Chemistry and Physics,2009,120(2):656-660.
【19】YANG L, ZHONG Z C, YOU J, et al. Acoustic emission evaluation of fracture characteristics in thermal barrier coatings under bending[J]. Surface&Coatings Technology, 2013, 232:710-718.
【20】WANG L,NI J X,SHAO F,et al.Failure behavior of plasma-sprayed yttria-stabilized zirconia thermal barrier coatings under three-point bending test via acoustic emission technique[J].Journal of Thermal Spray Technology,2017,26(1/2):116-131.
【21】李雪换,底月兰,王海斗,等.基于声发射技术的热障涂层拉伸失效模式研究[J].机械工程学报,2020,56(14):57-64. LI X H,DI Y L,WANG H D,et al.Research on crack failure modes of thermal barrier coatings based on acoustic emission technique[J].Journal of Mechanical Engineering,2020,56(14):57-64.
【22】李正阳,刘睿睿,张伟,等.工作电压对N36锆合金表面微弧氧化涂层磨蚀性能的影响[J].摩擦学学报,2021,41(6):880-889. LI Z Y,LIU R R,ZHANG W,et al.Effect of voltage on fretting corrosion behavior of micro-arc oxidation coating on N36 zirconium alloy[J].Tribology,2021,41(6):880-889.
【23】魏克俭,薛文斌,曲尧,等.锆微弧氧化表面处理技术研究进展[J].表面技术,2019,48(7):11-23. WEI K J,XUE W B,QU Y,et al.Advance in microarc oxidation surface treatment on Zr[J].Surface Technology,2019,48(7):11-23.
【24】LI Z Y,CAI Z B,CUI Y,et al.Effect of oxidation time on the impact wear of micro-arc oxidation coating on aluminum alloy[J].Wear,2019,426/427:285-295.
【25】WANG Z H,WU X,LIU X Q,et al.Research on feature extraction algorithm of rolling bearing fatigue evolution stage based on acoustic emission[J].Mechanical Systems and Signal Processing,2017,113:271-284.
【26】王昱,陈乐,陈寰,等.锆合金管表面Cr涂层的室温与高温拉伸性能研究[J].材料保护,2020,53(7):61-66. WANG Y,CHEN L,CHEN H,et al.Room and high temperature tensile properties of Cr coating on zircaloy tubes[J].Materials Protection,2020,53(7):61-66.
【27】AGRAWAL D C,RAJ R.Measurement of the ultimate shear strength of a metal-ceramic interface[J].Acta Metallurgica,1989,37(4):1265-1270.
【2】张强,齐世锋,陈鸿飞,等.在高温硝酸与丙烷蒸气环境中R60702工业纯锆的腐蚀行为[J].机械工程材料,2020,44(7):33-37. ZHANG Q,QI S F,CHEN H F,et al.Corrosion behavior of R60702 industrial pure zirconium in high temperature nitric acid and propane vapor[J].Materials for Mechanical Engineering,2020,44(7):33-37.
【3】MOTTA A T, YILMAZBAYHAN A, SILVA M J G D, et al. Zirconium alloys for supercritical water reactor applications:Challenges and possibilities[J]. Journal of Nuclear Materials, 2007, 371(1/2/3):61-75.
【4】GHOSAL S K, PALIT G C, DE P K. Corrosion of zirconium alloys in nuclear applications-A review[J]. Mineral Processing&Extractive Metallurgy Review, 2002, 22(4/5/6):519-546.
【5】NOUDURU S K, MANDAPAKA K K, ROYCHOWDHURY S, et al. Nodular corrosion of zirconium alloys in gaseous environment containing different contaminants[J]. Journal of Nuclear Materials, 2020, 545:152640.
【6】LI Z Y, CAI Z B, CUI X J, et al. Influence of nanoparticle additions on structure and fretting corrosion behavior of micro-arc oxidation coatings on zirconium alloy[J]. Surface and Coatings Technology, 2021, 410:126949.
【7】BRACHET J C, SAUX M L, BISCHOFF J, et al. Evaluation of equivalent cladding reacted parameters of Cr-coated claddings oxidized in steam at 1200℃ in relation with oxygen diffusion/partitioning and post-quench ductility[J]. Journal of Nuclear Materials, 2020,533:152106.
【8】BRAGG-SITTON S. Development of advanced accident tolerant fuels for commercial light water reactors[J]. Nuclear News, 2014, 57(3):83-91.
【9】CHEN H, WANG X, ZHANG R. Application and development progress of Cr-based surface coating in nuclear fuel elements:II. Current status and shortcomings of performance studies[J]. Coatings, 2020, 10(9):835-835.
【10】TANG C, STUEBER M, SEIFERT H J, et al. Protective coatings on zirconium-based alloys as accident-tolerant fuel (ATF) claddings[J]. Corrosion Reviews, 2017, 35(3):141-165.
【11】王晓云,马一林,田林海,等.Al2O3掺杂与超声辅助对纯铝表面微弧氧化层结构与性能的影响[J].机械工程材料,2018,42(11):52-57. WANG X Y,MA Y L,TIAN L H,et al.Effect of Al2O3 doping and ultrasonic assisting on structure and properties of micro-arc oxidation coating on surface of pure aluminum[J].Materials for Mechanical Engineering,2018,42(11):52-57.
【12】LIU F,SHAN D Y,SONG Y W,et al.Corrosion behavior of the composite ceramic coating containing zirconium oxides on AM30 magnesium alloy by plasma electrolytic oxidation[J].Corrosion Science,2011,53(11):3845-3852.
【13】XUE W,WANG C,TIALN H,et al.Corrosion behaviors and galvanic studies of microarc oxidation films on Al-Zn-Mg-Cu alloy[J].Surface&Coatings Technology,2007,201(21):8695-8701.
【14】WANG Y M,JIANG B L,GUO L X,et al.Tribological behavior of microarc oxidation coatings formed on titanium alloys against steel in dry and solid lubrication sliding[J].Applied Surface Science,2006,252(8):2989-2998.
【15】CHENG Y L,CAO J H,PENG Z M,et al.Wear-resistant coatings formed on zircaloy-2 by plasma electrolytic oxidation in sodium aluminate electrolytes[J].Electrochimica Acta,2014,116:453-466.
【16】YANG J, WANG X, WEN Q, et al. The effect of microarc oxidation and excimer laser processing on the microstructure and corrosion resistance of Zr-1Nb alloy[J]. Journal of Nuclear Materials, 2015, 467:186-193.
【17】MATYKINA E, ARRABAL R, SKELDON P, et al. Investigation of the growth processes of coatings formed by AC plasma electrolytic oxidation of aluminium[J]. Electrochimica Acta, 2009, 54(27):6767-6778.
【18】XUE W B,ZHU Q Z,JIN Q,et al.Characterization of ceramic coatings fabricated on zirconium alloy by plasma electrolytic oxidation in silicate electrolyte[J].Materials Chemistry and Physics,2009,120(2):656-660.
【19】YANG L, ZHONG Z C, YOU J, et al. Acoustic emission evaluation of fracture characteristics in thermal barrier coatings under bending[J]. Surface&Coatings Technology, 2013, 232:710-718.
【20】WANG L,NI J X,SHAO F,et al.Failure behavior of plasma-sprayed yttria-stabilized zirconia thermal barrier coatings under three-point bending test via acoustic emission technique[J].Journal of Thermal Spray Technology,2017,26(1/2):116-131.
【21】李雪换,底月兰,王海斗,等.基于声发射技术的热障涂层拉伸失效模式研究[J].机械工程学报,2020,56(14):57-64. LI X H,DI Y L,WANG H D,et al.Research on crack failure modes of thermal barrier coatings based on acoustic emission technique[J].Journal of Mechanical Engineering,2020,56(14):57-64.
【22】李正阳,刘睿睿,张伟,等.工作电压对N36锆合金表面微弧氧化涂层磨蚀性能的影响[J].摩擦学学报,2021,41(6):880-889. LI Z Y,LIU R R,ZHANG W,et al.Effect of voltage on fretting corrosion behavior of micro-arc oxidation coating on N36 zirconium alloy[J].Tribology,2021,41(6):880-889.
【23】魏克俭,薛文斌,曲尧,等.锆微弧氧化表面处理技术研究进展[J].表面技术,2019,48(7):11-23. WEI K J,XUE W B,QU Y,et al.Advance in microarc oxidation surface treatment on Zr[J].Surface Technology,2019,48(7):11-23.
【24】LI Z Y,CAI Z B,CUI Y,et al.Effect of oxidation time on the impact wear of micro-arc oxidation coating on aluminum alloy[J].Wear,2019,426/427:285-295.
【25】WANG Z H,WU X,LIU X Q,et al.Research on feature extraction algorithm of rolling bearing fatigue evolution stage based on acoustic emission[J].Mechanical Systems and Signal Processing,2017,113:271-284.
【26】王昱,陈乐,陈寰,等.锆合金管表面Cr涂层的室温与高温拉伸性能研究[J].材料保护,2020,53(7):61-66. WANG Y,CHEN L,CHEN H,et al.Room and high temperature tensile properties of Cr coating on zircaloy tubes[J].Materials Protection,2020,53(7):61-66.
【27】AGRAWAL D C,RAJ R.Measurement of the ultimate shear strength of a metal-ceramic interface[J].Acta Metallurgica,1989,37(4):1265-1270.
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